IndiumV3, Main, Repository, bibRecord, 000843

New rare-earth quinolinate complexes for organic light-emitting devices

Identifieur interne : 000843 ( Main/Repository ); précédent : 000842; suivant : 000844

New rare-earth quinolinate complexes for organic light-emitting devices

Auteurs : RBID : Pascal:13-0162240

Descripteurs français

Pascal (Inist)
- Diode électroluminescente organique, Propriété thermique, Stabilité thermique, Propriété optique, Propriété électrique, Diode électroluminescente, Quinoléine, Couche mince, Vide poussé, Evaporation, Oxyde d'étain, Couche oxyde, Diamine, Conductivité type p, Complexe de lanthanide, Aluminium, Composé de l'aluminium, Dérivé de la quinoléine, Oxyde d'indium, Electroluminescence, Ligand, Photoluminescence, Substrat silicium, Substrat quartz, 8560D, 6860D, 7866, 7350.
Wicri :
- concept : Aluminium.

English descriptors

KwdEn :
- Aluminium, Aluminium compound, Diamine, Electrical properties, Electroluminescence, Evaporation, High vacuum, Indium oxide, Ligand, Light emitting diode, Optical properties, Organic light emitting diodes, Oxide layer, P type conductivity, Photoluminescence, Quinoline, Quinoline derivatives, Rare earth metal complex, Thermal properties, Thermal stability, Thin film, Tin oxide.

Abstract

Because of its thermal and morphological stability and optical and electrical properties, tris(8-hydroxyquinoline) aluminum (Alq₃) is one of the most widely used electron transporting materials in organic light-emitting devices (OLEDs). The search for substitutes for this compound constitutes an important field of research in organic electronics. We report on a study of a new rare-earth tetrakis 8-hydroxyquinoline complex. Synthesis of tris complexes with rare-earth metals and 8-hydroxyquinoline resulted in unstable compounds. However, the inclusion of an additional quinoline group stabilized these compounds. Li[RE(q)₄] (where RE=La³⁺,Lu³⁺ and Y³⁺ and q = 8-hydroxyquinoline) were synthesized and then used as the electron-transporting and emitting layer in OLEDs. Thin films were deposited in a high-vacuum environment by thermal evaporation on quartz and silicon substrates. Optical characterization of the RE complexes revealed emission in the 510-525 nm range, the same as that observed for Alq₃, while absorption was observed at wavelengths of 382 nm for the Y/La complexes and 388 nm for the Lu complex. The OLEDs were fabricated with an indium tin oxide layer (ITO) as the anode, (N,N'-bis (1-naphtyl)-N,N'-diphenyl-1,1'-biphenyl-4,4'-diamine) NPB as the hole-transporting layer (25 nm), Li[RE(q)₄] as the electron-transporting and emitting layer (40 nm) and aluminum as the cathode (120 nm). The electroluminescence (EL) spectra showed a broad band from 520 to 540 nm and green-colored emission associated with the 8-hydroxyquinoline ligand. There was an interesting dependence of the maximum energy peak position and half-width of the emission band in the EL spectra on the atomic radius of the RE ion used. The best luminance for the OLEDs produced in this study was achieved with the Li[RE(q)₄] compound. The optical and electrical properties of this OLED were comparable to those of similar devices based on Alq₃.

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Pascal:13-0162240

Le document en format XML

<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en" level="a">New rare-earth quinolinate complexes for organic light-emitting devices</title>
<author><name sortKey="Camargo, H" uniqKey="Camargo H">H. Camargo</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Physics Department, Pontifical Catholic University of Rio de Janeiro</s1>
<s2>22453-900 Rio de Janeiro</s2>
<s3>BRA</s3>
<sZ>1 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>5 aut.</sZ>
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<country>Brésil</country>
<wicri:noRegion>22453-900 Rio de Janeiro</wicri:noRegion>
</affiliation>
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<author><name sortKey="Paolini, T B" uniqKey="Paolini T">T. B. Paolini</name>
<affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Chemistry Institute, Department of Fundamental Chemistry, University of São Paulo, USP</s1>
<s2>05599-970 São Paulo</s2>
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<country>Brésil</country>
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<author><name sortKey="Niyama, E" uniqKey="Niyama E">E. Niyama</name>
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<sZ>1 aut.</sZ>
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<author><name sortKey="Brito, H F" uniqKey="Brito H">H. F. Brito</name>
<affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Chemistry Institute, Department of Fundamental Chemistry, University of São Paulo, USP</s1>
<s2>05599-970 São Paulo</s2>
<s3>BRA</s3>
<sZ>2 aut.</sZ>
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<author><name sortKey="Cremona, M" uniqKey="Cremona M">M. Cremona</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Physics Department, Pontifical Catholic University of Rio de Janeiro</s1>
<s2>22453-900 Rio de Janeiro</s2>
<s3>BRA</s3>
<sZ>1 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>5 aut.</sZ>
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<country>Brésil</country>
<wicri:noRegion>22453-900 Rio de Janeiro</wicri:noRegion>
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<title level="j" type="main">Thin solid films</title>
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<term>Aluminium compound</term>
<term>Diamine</term>
<term>Electrical properties</term>
<term>Electroluminescence</term>
<term>Evaporation</term>
<term>High vacuum</term>
<term>Indium oxide</term>
<term>Ligand</term>
<term>Light emitting diode</term>
<term>Optical properties</term>
<term>Organic light emitting diodes</term>
<term>Oxide layer</term>
<term>P type conductivity</term>
<term>Photoluminescence</term>
<term>Quinoline</term>
<term>Quinoline derivatives</term>
<term>Rare earth metal complex</term>
<term>Thermal properties</term>
<term>Thermal stability</term>
<term>Thin film</term>
<term>Tin oxide</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Diode électroluminescente organique</term>
<term>Propriété thermique</term>
<term>Stabilité thermique</term>
<term>Propriété optique</term>
<term>Propriété électrique</term>
<term>Diode électroluminescente</term>
<term>Quinoléine</term>
<term>Couche mince</term>
<term>Vide poussé</term>
<term>Evaporation</term>
<term>Oxyde d'étain</term>
<term>Couche oxyde</term>
<term>Diamine</term>
<term>Conductivité type p</term>
<term>Complexe de lanthanide</term>
<term>Aluminium</term>
<term>Composé de l'aluminium</term>
<term>Dérivé de la quinoléine</term>
<term>Oxyde d'indium</term>
<term>Electroluminescence</term>
<term>Ligand</term>
<term>Photoluminescence</term>
<term>Substrat silicium</term>
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<term>8560D</term>
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<front><div type="abstract" xml:lang="en">Because of its thermal and morphological stability and optical and electrical properties, tris(8-hydroxyquinoline) aluminum (Alq<sub>3</sub>
) is one of the most widely used electron transporting materials in organic light-emitting devices (OLEDs). The search for substitutes for this compound constitutes an important field of research in organic electronics. We report on a study of a new rare-earth tetrakis 8-hydroxyquinoline complex. Synthesis of tris complexes with rare-earth metals and 8-hydroxyquinoline resulted in unstable compounds. However, the inclusion of an additional quinoline group stabilized these compounds. Li[RE(q)<sub>4</sub>
] (where RE=La<sup>3+</sup>
,<sup> </sup>
Lu<sup>3+</sup>
 and Y<sup>3+</sup>
 and q = 8-hydroxyquinoline) were synthesized and then used as the electron-transporting and emitting layer in OLEDs. Thin films were deposited in a high-vacuum environment by thermal evaporation on quartz and silicon substrates. Optical characterization of the RE complexes revealed emission in the 510-525 nm range, the same as that observed for Alq<sub>3</sub>
, while absorption was observed at wavelengths of 382 nm for the Y/La complexes and 388 nm for the Lu complex. The OLEDs were fabricated with an indium tin oxide layer (ITO) as the anode, (N,N'-bis (1-naphtyl)-N,N'-diphenyl-1,1'-biphenyl-4,4'-diamine) NPB as the hole-transporting layer (25 nm), Li[RE(q)<sub>4</sub>
] as the electron-transporting and emitting layer (40 nm) and aluminum as the cathode (120 nm). The electroluminescence (EL) spectra showed a broad band from 520 to 540 nm and green-colored emission associated with the 8-hydroxyquinoline ligand. There was an interesting dependence of the maximum energy peak position and half-width of the emission band in the EL spectra on the atomic radius of the RE ion used. The best luminance for the OLEDs produced in this study was achieved with the Li[RE(q)<sub>4</sub>
] compound. The optical and electrical properties of this OLED were comparable to those of similar devices based on Alq<sub>3</sub>
.</div>
</front>
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<fA09 i1="01" i2="1" l="ENG"><s1>Proceedings of the 39th International Conference on Metallurgical Coatings and Thin Films (ICMCTF 2012), San Diego, California (USA), April 23-27, 2012</s1>
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<s9>ed.</s9>
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<s9>ed.</s9>
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<fA12 i1="05" i2="1"><s1>STÜBER (Michael)</s1>
<s9>ed.</s9>
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<fA12 i1="06" i2="1"><s1>VEPREK (Stan)</s1>
<s9>ed.</s9>
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<fA14 i1="01"><s1>Physics Department, Pontifical Catholic University of Rio de Janeiro</s1>
<s2>22453-900 Rio de Janeiro</s2>
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<sZ>1 aut.</sZ>
<sZ>3 aut.</sZ>
<sZ>5 aut.</sZ>
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<sZ>2 aut.</sZ>
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<fA15 i1="01"><s1>University of Poitiers - Institut P', Department Physique et Mécanique des Matériaux, SP2MI, Teleport 2, Bd. Marie et Pierre Curie</s1>
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<s3>FRA</s3>
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<fA15 i1="02"><s1>Southern Illinois University Carbondale, Department of Physics, 1245 Lincoln Drive, Neckers 483 A</s1>
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<s3>USA</s3>
<sZ>2 aut.</sZ>
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<fA15 i1="03"><s1>University of Cyprus, Mechanical & Manufacturing Engineering, 75 Kallipoleos Street</s1>
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<sZ>4 aut.</sZ>
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<fA15 i1="04"><s1>Karlsruhe Institute of Technology (KIT), Institute for Applied Materials (IAM), Hermann-von-Helmholtz-Platz 1</s1>
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<sZ>6 aut.</sZ>
</fA15>
<fA18 i1="01" i2="1"><s1>American Vacuum Society (AVS). Surface Engineering Division (ASED)</s1>
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<fC01 i1="01" l="ENG"><s0>Because of its thermal and morphological stability and optical and electrical properties, tris(8-hydroxyquinoline) aluminum (Alq<sub>3</sub>
) is one of the most widely used electron transporting materials in organic light-emitting devices (OLEDs). The search for substitutes for this compound constitutes an important field of research in organic electronics. We report on a study of a new rare-earth tetrakis 8-hydroxyquinoline complex. Synthesis of tris complexes with rare-earth metals and 8-hydroxyquinoline resulted in unstable compounds. However, the inclusion of an additional quinoline group stabilized these compounds. Li[RE(q)<sub>4</sub>
] (where RE=La<sup>3+</sup>
,<sup> </sup>
Lu<sup>3+</sup>
 and Y<sup>3+</sup>
 and q = 8-hydroxyquinoline) were synthesized and then used as the electron-transporting and emitting layer in OLEDs. Thin films were deposited in a high-vacuum environment by thermal evaporation on quartz and silicon substrates. Optical characterization of the RE complexes revealed emission in the 510-525 nm range, the same as that observed for Alq<sub>3</sub>
, while absorption was observed at wavelengths of 382 nm for the Y/La complexes and 388 nm for the Lu complex. The OLEDs were fabricated with an indium tin oxide layer (ITO) as the anode, (N,N'-bis (1-naphtyl)-N,N'-diphenyl-1,1'-biphenyl-4,4'-diamine) NPB as the hole-transporting layer (25 nm), Li[RE(q)<sub>4</sub>
] as the electron-transporting and emitting layer (40 nm) and aluminum as the cathode (120 nm). The electroluminescence (EL) spectra showed a broad band from 520 to 540 nm and green-colored emission associated with the 8-hydroxyquinoline ligand. There was an interesting dependence of the maximum energy peak position and half-width of the emission band in the EL spectra on the atomic radius of the RE ion used. The best luminance for the OLEDs produced in this study was achieved with the Li[RE(q)<sub>4</sub>
] compound. The optical and electrical properties of this OLED were comparable to those of similar devices based on Alq<sub>3</sub>
.</s0>
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<s5>09</s5>
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<s5>09</s5>
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<s5>10</s5>
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<s5>10</s5>
</fC03>
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<s5>10</s5>
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<s5>11</s5>
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<s5>12</s5>
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<s5>13</s5>
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<s5>15</s5>
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<s2>NC</s2>
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<s5>16</s5>
</fC03>
<fC03 i1="16" i2="X" l="ENG"><s0>Aluminium</s0>
<s2>NC</s2>
<s2>FR</s2>
<s2>FX</s2>
<s5>16</s5>
</fC03>
<fC03 i1="16" i2="X" l="SPA"><s0>Aluminio</s0>
<s2>NC</s2>
<s2>FR</s2>
<s2>FX</s2>
<s5>16</s5>
</fC03>
<fC03 i1="17" i2="X" l="FRE"><s0>Composé de l'aluminium</s0>
<s5>17</s5>
</fC03>
<fC03 i1="17" i2="X" l="ENG"><s0>Aluminium compound</s0>
<s5>17</s5>
</fC03>
<fC03 i1="17" i2="X" l="SPA"><s0>Aluminio compuesto</s0>
<s5>17</s5>
</fC03>
<fC03 i1="18" i2="X" l="FRE"><s0>Dérivé de la quinoléine</s0>
<s2>FF</s2>
<s5>18</s5>
</fC03>
<fC03 i1="18" i2="X" l="ENG"><s0>Quinoline derivatives</s0>
<s2>FF</s2>
<s5>18</s5>
</fC03>
<fC03 i1="18" i2="X" l="SPA"><s0>Quinolina derivado</s0>
<s2>FF</s2>
<s5>18</s5>
</fC03>
<fC03 i1="19" i2="X" l="FRE"><s0>Oxyde d'indium</s0>
<s5>19</s5>
</fC03>
<fC03 i1="19" i2="X" l="ENG"><s0>Indium oxide</s0>
<s5>19</s5>
</fC03>
<fC03 i1="19" i2="X" l="SPA"><s0>Indio óxido</s0>
<s5>19</s5>
</fC03>
<fC03 i1="20" i2="X" l="FRE"><s0>Electroluminescence</s0>
<s5>29</s5>
</fC03>
<fC03 i1="20" i2="X" l="ENG"><s0>Electroluminescence</s0>
<s5>29</s5>
</fC03>
<fC03 i1="20" i2="X" l="SPA"><s0>Electroluminiscencia</s0>
<s5>29</s5>
</fC03>
<fC03 i1="21" i2="X" l="FRE"><s0>Ligand</s0>
<s5>30</s5>
</fC03>
<fC03 i1="21" i2="X" l="ENG"><s0>Ligand</s0>
<s5>30</s5>
</fC03>
<fC03 i1="21" i2="X" l="SPA"><s0>Ligando</s0>
<s5>30</s5>
</fC03>
<fC03 i1="22" i2="X" l="FRE"><s0>Photoluminescence</s0>
<s5>31</s5>
</fC03>
<fC03 i1="22" i2="X" l="ENG"><s0>Photoluminescence</s0>
<s5>31</s5>
</fC03>
<fC03 i1="22" i2="X" l="SPA"><s0>Fotoluminiscencia</s0>
<s5>31</s5>
</fC03>
<fC03 i1="23" i2="X" l="FRE"><s0>Substrat silicium</s0>
<s4>INC</s4>
<s5>46</s5>
</fC03>
<fC03 i1="24" i2="X" l="FRE"><s0>Substrat quartz</s0>
<s4>INC</s4>
<s5>47</s5>
</fC03>
<fC03 i1="25" i2="X" l="FRE"><s0>8560D</s0>
<s4>INC</s4>
<s5>71</s5>
</fC03>
<fC03 i1="26" i2="X" l="FRE"><s0>6860D</s0>
<s4>INC</s4>
<s5>72</s5>
</fC03>
<fC03 i1="27" i2="X" l="FRE"><s0>7866</s0>
<s4>INC</s4>
<s5>73</s5>
</fC03>
<fC03 i1="28" i2="X" l="FRE"><s0>7350</s0>
<s4>INC</s4>
<s5>74</s5>
</fC03>
<fN21><s1>140</s1>
</fN21>
<fN44 i1="01"><s1>OTO</s1>
</fN44>
<fN82><s1>OTO</s1>
</fN82>
</pA>
<pR><fA30 i1="01" i2="1" l="ENG"><s1>ICMCTF 2012 International Conference on Metallurgical Coatings and Thin Films</s1>
<s2>39</s2>
<s3>San Diego, California USA</s3>
<s4>2012-04-23</s4>
</fA30>
</pR>
</standard>
</inist>
</record>

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   |texte=   New rare-earth quinolinate complexes for organic light-emitting devices
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New rare-earth quinolinate complexes for organic light-emitting devices

New rare-earth quinolinate complexes for organic light-emitting devices

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